The concept that superconductivity competes with other orders in cuprate superconductors has become increasingly apparent, but obtaining direct evidence with bulk-sensitive probes is challenging. We have used resonant soft x-ray scattering to identify two-dimensional charge fluctuations with an incommensurate periodicity of ~3.2 lattice units in the copper-oxide planes of the superconductors (Y,Nd)Ba(2)Cu(3)O(6+)(x), with hole concentrations of 0.09 to 0.13 per planar Cu ion. The intensity and correlation length of the fluctuation signal increase strongly upon cooling down to the superconducting transition temperature (T(c)); further cooling below T(c) abruptly reverses the divergence of the charge correlations. In combination with earlier observations of a large gap in the spin excitation spectrum, these data indicate an incipient charge density wave instability that competes with superconductivity.
Long-range incommensurate charge fluctuations in (Y,Nd)Ba2Cu3O6+x / Ghiringhelli, G.; Le Tacon, M.; Minola, M.; Blanco-Canosa, S.; Mazzoli, C.; Brookes, N. B.; De Luca, G. M.; Frano, A.; Hawthorn, D. G.; He, F.; Loew, T.; Moretti Sala, M.; Peets, D. C.; Salluzzo, M.; Schierle, E.; Sutarto, R.; Sawatzky, G. A.; Weschke, E.; Keimer, B.; Braicovich, L.. - In: SCIENCE. - ISSN 0036-8075. - 337:6096(2012), pp. 821-825. [10.1126/science.1223532]
Long-range incommensurate charge fluctuations in (Y,Nd)Ba2Cu3O6+x
Ghiringhelli G.;De Luca G. M.;He F.;
2012
Abstract
The concept that superconductivity competes with other orders in cuprate superconductors has become increasingly apparent, but obtaining direct evidence with bulk-sensitive probes is challenging. We have used resonant soft x-ray scattering to identify two-dimensional charge fluctuations with an incommensurate periodicity of ~3.2 lattice units in the copper-oxide planes of the superconductors (Y,Nd)Ba(2)Cu(3)O(6+)(x), with hole concentrations of 0.09 to 0.13 per planar Cu ion. The intensity and correlation length of the fluctuation signal increase strongly upon cooling down to the superconducting transition temperature (T(c)); further cooling below T(c) abruptly reverses the divergence of the charge correlations. In combination with earlier observations of a large gap in the spin excitation spectrum, these data indicate an incipient charge density wave instability that competes with superconductivity.File | Dimensione | Formato | |
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