Dynamic wire-pull rubber diaphragm for rapid formation and spatio-temporal investigation of multi-shape free-standing liquid films

Quantitative manufacturing and characterization of thin films are relevant in different scientific and industrial fields. Especially, for the studies of fluid dynamics, the experimental verification of theoretical models creates the need of a free-standing liquid film formation. Driven by the lack of fast and accurate liquid film forming technology, we present a novel device able to fabricate thin free-standing liquid films, which is based on a dynamic and adjustable diaphragm, the opening of which allows for the rapid formation of a self-supported liquid film confined in a wire-pull rubber band. The quantitative thickness mapping of the film formation and its time- resolved evolution are performed by digital holography in real-time. This builds up a strategy that allows for the accurate liquid film formation with controllable size and volume. As the results, multi-shape and multi- material thin films under controllable and stable conditions are successfully formed, including free-standing water, soapy water and glycerol films. A label-free spatio-temporal analysis method for flow dynamics is proposed: The full-field time series of film thickness is reassembled in a new coordinate system composed of radius, time, and thickness. Such spatio-temporal analysis reveals details of leveling and drainage processes. To the best of our knowledge, this is the first full-field quantitative thickness analysis of multi-shape and multi-material thin films. The proposed Dynamic Wire-pull Rubber Diaphragm (DWRD) together with the digital holography add-on offer characterization abilities with an unprecedented level of details allowing for a deeper understanding of the underlying thin film dynamics that can be useful in several different scientific and technological fields as biotechnology, life science, and nanotechnology.